Definition of unrelaxed
: not at rest or at ease : not relaxed
… the more rattled and unrelaxed he gets.— Maureen Dowd … the moon gazed on my midnight labours, while, with unrelaxed and breathless eagerness, I pursued nature to her hiding-places.— Mary Shelley
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Merriam-Webster unabridged
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Time Traveler for unrelaxed
The first known use of unrelaxed was in 1508
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